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Ce(IV)- and HClO(4)-Promoted Assembly of an Fe(2)(IV)(μ-O)(2) Diamond Core from its Monomeric Fe(IV)=O Precursor at Room Temperature

Diiron(IV)-oxo species are proposed to effect the cleavage of strong C–H bonds by nonheme diiron enzymes such as soluble methane monooxygenase (sMMO) and fatty acid desaturases. However, synthetic mimics of such diiron(IV) oxidants are rare. Herein we report the reaction of (TPA*)Fe(II) (1) (TPA* =...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Draksharapu, Apparao, Xu, Shuangning, Que, Lawrence
Formato: Artigo
Idioma:Inglês
Publicado em: 2020
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7708462/
https://ncbi.nlm.nih.gov/pubmed/32902902
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.202010027
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