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Ce(IV)- and HClO(4)-Promoted Assembly of an Fe(2)(IV)(μ-O)(2) Diamond Core from its Monomeric Fe(IV)=O Precursor at Room Temperature

Diiron(IV)-oxo species are proposed to effect the cleavage of strong C–H bonds by nonheme diiron enzymes such as soluble methane monooxygenase (sMMO) and fatty acid desaturases. However, synthetic mimics of such diiron(IV) oxidants are rare. Herein we report the reaction of (TPA*)Fe(II) (1) (TPA* =...

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Vydáno v:Angew Chem Int Ed Engl
Hlavní autoři: Draksharapu, Apparao, Xu, Shuangning, Que, Lawrence
Médium: Artigo
Jazyk:Inglês
Vydáno: 2020
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On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC7708462/
https://ncbi.nlm.nih.gov/pubmed/32902902
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.202010027
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