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Million-fold activation of the [Fe(2)(μ-O)(2)] diamond core for C-H bond cleavage

In biological systems, the cleavage of strong C–H bonds is often carried out by iron centers – such as the methane monooxygenase in methane hydroxylation – through dioxygen activation mechanisms. High valent species with [Fe(2)(μ-O)(2)] diamond cores are thought to act as the oxidizing moieties, but...

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Autors principals: Xue, Genqiang, De Hont, Raymond, Münck, Eckard, Que, Lawrence
Format: Artigo
Idioma:Inglês
Publicat: 2010
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Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC2859466/
https://ncbi.nlm.nih.gov/pubmed/20414242
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/nchem.586
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