Vibrational Perturbation of the [FeFe] Hydrogenase H-Cluster Revealed by (13)C(2)H-ADT Labeling

[FeFe] hydrogenases are highly active catalysts for the interconversion of molecular hydrogen with protons and electrons. Here, we use a combination of isotopic labeling, (57)Fe nuclear resonance vibrational spectroscopy (NRVS), and density functional theory (DFT) calculations to observe and charact...

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發表在:J Am Chem Soc
Main Authors: Pelmenschikov, Vladimir, Birrell, James A., Gee, Leland B., Richers, Casseday P., Reijerse, Edward J., Wang, Hongxin, Arragain, Simon, Mishra, Nakul, Yoda, Yoshitaka, Matsuura, Hiroaki, Li, Lei, Tamasaku, Kenji, Rauchfuss, Thomas B., Lubitz, Wolfgang, Cramer, Stephen P.
格式: Artigo
語言:Inglês
出版: 2021
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Article
在線閱讀:https://ncbi.nlm.nih.gov/pmc/articles/PMC8211414/
https://ncbi.nlm.nih.gov/pubmed/34043346
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.1c02323
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