Vibrational Perturbation of the [FeFe] Hydrogenase H-Cluster Revealed by (13)C(2)H-ADT Labeling

[FeFe] hydrogenases are highly active catalysts for the interconversion of molecular hydrogen with protons and electrons. Here, we use a combination of isotopic labeling, (57)Fe nuclear resonance vibrational spectroscopy (NRVS), and density functional theory (DFT) calculations to observe and charact...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Pelmenschikov, Vladimir, Birrell, James A., Gee, Leland B., Richers, Casseday P., Reijerse, Edward J., Wang, Hongxin, Arragain, Simon, Mishra, Nakul, Yoda, Yoshitaka, Matsuura, Hiroaki, Li, Lei, Tamasaku, Kenji, Rauchfuss, Thomas B., Lubitz, Wolfgang, Cramer, Stephen P.
Formato: Artigo
Idioma:Inglês
Publicado em: 2021
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Article
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC8211414/
https://ncbi.nlm.nih.gov/pubmed/34043346
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.1c02323
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