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Asymmetry in the Ligand Coordination Sphere of the [FeFe] Hydrogenase Active Site Is Reflected in the Magnetic Spin Interactions of the Aza-propanedithiolate Ligand
[Image: see text] [FeFe] hydrogenases are very active enzymes that catalyze the reversible conversion of molecular hydrogen into protons and electrons. Their active site, the H-cluster, contains a unique binuclear iron complex, [2Fe](H), with CN(–) and CO ligands as well as an aza-propane-dithiolate...
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| 發表在: | J Phys Chem Lett |
|---|---|
| Main Authors: | , , , , , , , |
| 格式: | Artigo |
| 語言: | Inglês |
| 出版: |
American Chemical
Society
2019
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| 在線閱讀: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6844125/ https://ncbi.nlm.nih.gov/pubmed/31580680 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.jpclett.9b02354 |
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