Reaction Coordinate Leading to H(2) Production in [FeFe]-Hydrogenase Identified by NRVS and DFT

[FeFe]-hydrogenases are metalloenzymes that reversibly reduce protons to molecular hydrogen at exceptionally high rates. We have characterized the catalytically competent hydride state (H(hyd)) in the [FeFe]-hydrogenases from both Chlamydomonas reinhardtii and Desulfovibrio desulfuricans using (57)F...

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Veröffentlicht in:J Am Chem Soc
Hauptverfasser: Pelmenschikov, Vladimir, Birrell, James A., Pham, Cindy C., Mishra, Nakul, Wang, Hongxin, Sommer, Constanze, Reijerse, Edward, Richers, Casseday P., Tamasaku, Kenji, Yoda, Yoshitaka, Rauchfuss, Thomas B., Lubitz, Wolfgang, Cramer, Stephen P.
Format: Artigo
Sprache:Inglês
Veröffentlicht: 2017
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Article
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC5699932/
https://ncbi.nlm.nih.gov/pubmed/29054130
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.7b09751
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