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Direct Observation of an Iron-Bound Terminal Hydride in [FeFe]-Hydrogenase by Nuclear Resonance Vibrational Spectroscopy
[FeFe]-hydrogenases catalyze the reversible reduction of protons to molecular hydrogen with extremely high efficiency. The active site (“H-cluster”) consists of a [4Fe–4S](H) cluster linked through a bridging cysteine to a [2Fe](H) subsite coordinated by CN(−) and CO ligands featuring a dithiol-amin...
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| Izdano u: | J Am Chem Soc |
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| Glavni autori: | , , , , , , , , , , , |
| Format: | Artigo |
| Jezik: | Inglês |
| Izdano: |
2017
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| Teme: | |
| Online pristup: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5545132/ https://ncbi.nlm.nih.gov/pubmed/28291336 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.7b00686 |
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