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Strong Inhibition of O-Atom Transfer Reactivity for Mn(IV)(O)(π-radical-cation)(Lewis acid) Versus Mn(V)(O) Porphyrinoid Complexes

The oxygen atom transfer (OAT) reactivity of two valence tautomers of a Mn(V)(O) porphyrinoid complex was compared. The OAT kinetics of Mn(V)(O)(TBP(8)Cz) (TBP(8)Cz = octakis(p-tert-butylphenyl)corrolazinato(3−)) reacting with a series of triarylphosphine (PAr(3)) substrates were monitored by stoppe...

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Bibliografske podrobnosti
izdano v:J Am Chem Soc
Main Authors: Zaragoza, Jan Paulo T., Baglia, Regina A., Siegler, Maxime A., Goldberg, David P.
Format: Artigo
Jezik:Inglês
Izdano: 2015
Teme:
Online dostop:https://ncbi.nlm.nih.gov/pmc/articles/PMC4888055/
https://ncbi.nlm.nih.gov/pubmed/25964988
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.5b00875
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