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Meso-N-methylation of a porphyrinoid complex: Activating the H-atom transfer capability of an inert Re(V)(O) corrolazine()

The selective alkylation of a single meso-N atom of a corrolazine macrocycle is reported. Alkylation has a dramatic impact on the physicochemical properties of Re(V)(O)(TBP(8)Cz). New electron-transfer and hydrogen-atom-transfer reactivity is also seen for this complex, including one-electron reduct...

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Detalhes bibliográficos
Publicado no:Chem Commun (Camb)
Main Authors: Joslin, Evan E., Zaragoza, Jan Paulo T., Siegler, Maxime A., Goldberg, David P.
Formato: Artigo
Idioma:Inglês
Publicado em: 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5351293/
https://ncbi.nlm.nih.gov/pubmed/28119963
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c6cc09341h
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