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Mechanistic Studies of the Radical SAM Enzyme DesII with TDP-d-Fucose

DesII is a radical SAM enzyme that catalyzes the C4-deamination of TDP-4-amino-4,6-dideoxyglucose via a C3 radical intermediate. However, if the C4 amino group is replaced with a hydroxyl (TDP-quinovose), the hydroxyl at C3 is oxidized to a ketone with no C4-dehydration. It is hypothesized that hype...

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Bibliografiset tiedot
Julkaisussa:Angew Chem Int Ed Engl
Päätekijät: Ko, Yeonjin, Ruszczycky, Mark W., Choi, Sei-Hyun, Liu, Hung-wen
Aineistotyyppi: Artigo
Kieli:Inglês
Julkaistu: 2014
Aiheet:
Linkit:https://ncbi.nlm.nih.gov/pmc/articles/PMC4293265/
https://ncbi.nlm.nih.gov/pubmed/25418063
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201409540
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