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Photoenzymatic Catalysis Enables Radical-Mediated Ketone Reduction in ‘Ene’-Reductases

Flavin-dependent ‘ene’-reductases (EREDs) are known to stereoselectively reduce activated alkenes, but are inactive toward carbonyls. Herein we demonstrate that in the presence of photoredox catalysts, these enzymes will reduce aromatic ketones. Mechanistic experiments suggest this reaction proceeds...

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Bibliografiska uppgifter
I publikationen:Angew Chem Int Ed Engl
Huvudupphovsmän: Sandoval, Braddock A., Kurtoic, Sarah I., Chung, Megan M., Biegasiewicz, Kyle F., Hyster, Todd K.
Materialtyp: Artigo
Språk:Inglês
Publicerad: 2019
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Länkar:https://ncbi.nlm.nih.gov/pmc/articles/PMC6570536/
https://ncbi.nlm.nih.gov/pubmed/30951226
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201902005
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