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Photoenzymatic Generation of Unstabilized Alkyl Radicals: An Asymmetric Reductive Cyclization

Flavin-dependent ‘ene’-reductases (ERED) can generate stabilized alkyl radicals when irradiated with visible light, however, they are not known to form unstabilized radicals. Here, we report an enantioselective radical cyclization using alkyl iodides as precursors to unstabilized nucleophilic radica...

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Publicat a:J Am Chem Soc
Autors principals: Clayman, Phillip D., Hyster, Todd K.
Format: Artigo
Idioma:Inglês
Publicat: 2020
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC7778473/
https://ncbi.nlm.nih.gov/pubmed/32857506
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.0c07918
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