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Enantioselective Synthesis of Chiral Cyclopent‐2‐enones by Nickel‐Catalyzed Desymmetrization of Malonate Esters

The enantioselective synthesis of highly functionalized chiral cyclopent‐2‐enones by the reaction of alkynyl malonate esters with arylboronic acids is described. These desymmetrizing arylative cyclizations are catalyzed by a chiral phosphinooxazoline/nickel complex, and cyclization is enabled by the...

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Bibliografiske detaljer
Udgivet i:Angew Chem Int Ed Engl
Main Authors: Karad, Somnath Narayan, Panchal, Heena, Clarke, Christopher, Lewis, William, Lam, Hon Wai
Format: Artigo
Sprog:Inglês
Udgivet: John Wiley and Sons Inc. 2018
Fag:
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC6485403/
https://ncbi.nlm.nih.gov/pubmed/29768708
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201805578
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