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Enantioselective Synthesis of Chiral Cyclopent‐2‐enones by Nickel‐Catalyzed Desymmetrization of Malonate Esters

The enantioselective synthesis of highly functionalized chiral cyclopent‐2‐enones by the reaction of alkynyl malonate esters with arylboronic acids is described. These desymmetrizing arylative cyclizations are catalyzed by a chiral phosphinooxazoline/nickel complex, and cyclization is enabled by the...

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Detalles Bibliográficos
Publicado en:Angew Chem Int Ed Engl
Main Authors: Karad, Somnath Narayan, Panchal, Heena, Clarke, Christopher, Lewis, William, Lam, Hon Wai
Formato: Artigo
Idioma:Inglês
Publicado: John Wiley and Sons Inc. 2018
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Acceso en liña:https://ncbi.nlm.nih.gov/pmc/articles/PMC6485403/
https://ncbi.nlm.nih.gov/pubmed/29768708
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201805578
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