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Kinetic Understanding of N(2) Reduction versus H(2) Evolution at the E(4)(4H) Janus State in the Three Nitrogenases
The enzyme nitrogenase catalyzes the reduction of N(2) to ammonia but also that of protons to H(2). These reactions compete at the mechanistically central ‘Janus’ intermediate, denoted E(4)(4H), which has accumulated 4e(−)/4H(+) as two bridging Fe-H—Fe hydrides on the active-site cofactor. This stat...
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| Udgivet i: | Biochemistry |
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| Main Authors: | , , , , |
| Format: | Artigo |
| Sprog: | Inglês |
| Udgivet: |
2018
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| Fag: | |
| Online adgang: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6459397/ https://ncbi.nlm.nih.gov/pubmed/30183278 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.biochem.8b00784 |
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