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Photoinduced Reductive Elimination of H(2) from the Nitrogenase Dihydride (Janus) State Involves a FeMo-cofactor-H(2) Intermediate

N(2) reduction by nitrogenase involves the accumulation of four reducing equivalents at the active site FeMo-cofactor to form a state with two [Fe-H-Fe] bridging hydrides (denoted E(4)(4H), the Janus intermediate), and we recently demonstrated that the enzyme is activated to cleave the N≡N triple bo...

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Detalhes bibliográficos
Publicado no:Inorg Chem
Main Authors: Lukoyanov, Dmitriy, Khadka, Nimesh, Dean, Dennis R., Raugei, Simone, Seefeldt, Lance C., Hoffman, Brian M.
Formato: Artigo
Idioma:Inglês
Publicado em: 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5444871/
https://ncbi.nlm.nih.gov/pubmed/28177622
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.inorgchem.6b02899
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