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Highly Diastereo- and Enantioselective Synthesis of Nitrile-Substituted Cyclopropanes by Myoglobin-Mediated Carbene Transfer Catalysis

A chemobiocatalytic strategy for the highly stereoselective synthesis of nitrile-substituted cyclopropanes is reported. The present approach relies on an asymmetric olefin cyclopropanation reaction catalyzed by an engineered myoglobin in the presence of ex situ generated diazoacetonitrile within a c...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Chandgude, Ajay L., Fasan, Rudi
Formato: Artigo
Idioma:Inglês
Publicado em: 2018
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6436623/
https://ncbi.nlm.nih.gov/pubmed/30300955
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201810059
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