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Stereodivergent Intramolecular Cyclopropanation Enabled by Engineered Carbene Transferases
We report the development of engineered myoglobin biocatalysts for executing asymmetric intramolecular cyclopropanations resulting in cyclopropane-fused γ-lactones, which are key motifs found in many bioactive molecules. Using this strategy, a broad range of allyl diazoacetate substrates were effici...
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| Publicado no: | J Am Chem Soc |
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| Main Authors: | , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2019
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6561828/ https://ncbi.nlm.nih.gov/pubmed/31099569 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b02700 |
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