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Substrate and Lewis Acid Coordination Promote O–O Bond Cleavage of an Unreactive L(2)Cu(II)(2)(O(2)(2−)) Species to Form L(2)Cu(III)(2)(O)(2) Cores with Enhanced Oxidative Reactivity
Copper-dependent metalloenzymes are widespread throughout metabolic pathways, coupling the reduction of O(2) with the oxidation of organic substrates. Small-molecule synthetic analogs are useful platforms to generate L/Cu/O(2) species that reproduce the structural, spectroscopic, and reactive proper...
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| Publicado no: | J Am Chem Soc |
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| Main Authors: | , , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2017
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5532877/ https://ncbi.nlm.nih.gov/pubmed/28195739 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b12990 |
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