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An organometallic complex formed by an unconventional radical SAM enzyme

Pyrococcus horikoshii Dph2 (PhDph2) is an unusual radical SAM enzyme involved in the first step of diphthamide biosynthesis. It catalyzes the reaction by cleaving S-adenosylmethionine (SAM) to generate a 3-amino-3-carboxy propyl (ACP) radical. To probe the reaction mechanism, we synthesized a SAM an...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Dong, Min, Horitani, Masaki, Dzikovski, Boris, Pandelia, Maria-Eirini, Krebs, Carsten, Freed, Jack H., Hoffman, Brian, Lin, Hening
Formato: Artigo
Idioma:Inglês
Publicado em: 2016
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5068486/
https://ncbi.nlm.nih.gov/pubmed/27465315
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b04155
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