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Radical SAM Enzyme Spore Photoproduct Lyase: Properties of the Ω Organometallic Intermediate and Identification of Stable Protein Radicals Formed during Substrate-Free Turnover
Spore photoproduct lyase is a radical S-adenosyl-l-methionine (SAM) enzyme with the unusual property that addition of SAM to the [4Fe-4S](1+) enzyme absent substrate results in rapid electron transfer to SAM with accompanying homolytic S─C5′ bond cleavage. Herein, we demonstrate that this unusual re...
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| Publicado no: | J Am Chem Soc |
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| Main Authors: | , , , , , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2020
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC7730139/ https://ncbi.nlm.nih.gov/pubmed/32966073 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.0c08585 |
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