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(4+1) vs (4+2): Catalytic Intramolecular Coupling between Cy-clobutanones and Trisubstituted Allenes via C–C Activation

Herein we describe a rhodium-catalyzed (4+1) cyclization between cyclobutanones and allenes, which provides a distinct [4.2.1]-bicyclic skeleton containing two quaternary carbon centers. The reaction involves C–C activation of cyclobutanones and employs allenes as a one-carbon unit. A variety of fun...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Zhou, Xuan, Dong, Guangbin
Formato: Artigo
Idioma:Inglês
Publicado em: 2015
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4884657/
https://ncbi.nlm.nih.gov/pubmed/26440740
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.5b09799
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