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Total Synthesis of Cryptocaryol A via Enantioselective Iridium Catalyzed Alcohol C-H Allylation()

The polyketide natural product Cryptocaryol A is prepared in 8 steps via iridium catalyzed enantioselective diol double C-H allylation, which directly generates an acetate-based triketide stereodiad. In 4 previously reported total syntheses, 17-28 steps were required. [Image: see text]

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Foilsithe in:Angew Chem Int Ed Engl
Main Authors: Perez, Felix, Waldeck, Andrew R., Krische, Michael J.
Formáid: Artigo
Teanga:Inglês
Foilsithe: 2016
Ábhair:
Rochtain Ar Líne:https://ncbi.nlm.nih.gov/pmc/articles/PMC4834877/
https://ncbi.nlm.nih.gov/pubmed/27079820
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201600591
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