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(19)F NMR and DFT Analysis Reveal Structural and Electronic Transition State Features for RhoA‐Catalyzed GTP Hydrolysis
Molecular details for RhoA/GAP catalysis of the hydrolysis of GTP to GDP are poorly understood. We use (19)F NMR chemical shifts in the MgF(3) (−) transition state analogue (TSA) complex as a spectroscopic reporter to indicate electron distribution for the γ‐PO(3) (−) oxygens in the corresponding TS...
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| Publicado no: | Angew Chem Int Ed Engl |
|---|---|
| Main Authors: | , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
John Wiley and Sons Inc.
2016
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC4770445/ https://ncbi.nlm.nih.gov/pubmed/26822702 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201509477 |
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