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Substrate positioning controls the partition between halogenation and hydroxylation in the aliphatic halogenase, SyrB2
The α-ketoglutarate-dependent hydroxylases and halogenases employ similar reaction mechanisms involving hydrogen-abstracting Fe(IV)-oxo (ferryl) intermediates. In the halogenases, the carboxylate residue from the His(2)(Asp/Glu)(1)“facial triad” of iron ligands found in the hydroxylases is replaced...
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Main Authors: | , , , , , , , |
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Formato: | Artigo |
Idioma: | Inglês |
Publicado em: |
National Academy of Sciences
2009
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Assuntos: | |
Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC2764930/ https://ncbi.nlm.nih.gov/pubmed/19815524 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.0909649106 |
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