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Electronic Structure of the Ferryl Intermediate in the α-Ketoglutarate Dependent Non-Heme Iron Halogenase SyrB2: Contributions to H Atom Abstraction Reactivity

Low temperature magnetic circular dichroism (LT MCD) spectroscopy in combination with quantum-chemical calculations are used to define the electronic structure associated with the geometric structure of the Fe(IV)═O intermediate in SyrB2 that was previously determined by nuclear resonance vibrationa...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Srnec, Martin, Wong, Shaun D., Matthews, Megan L., Krebs, Carsten, Bollinger, J. Martin, Solomon, Edward I.
Formato: Artigo
Idioma:Inglês
Publicado em: 2016
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC4927264/
https://ncbi.nlm.nih.gov/pubmed/27021969
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b01151
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