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Mechanistic Insight into N=N Cleavage by a Low-Coordinate Iron(II) Hydride Complex

The reaction pathways of high-spin iron hydride complexes are relevant to the mechanism of N(2) reduction by nitrogenase, which has been postulated to involve paramagnetic iron-hydride species. However, almost all known iron hydrides are low-spin, diamagnetic Fe(II) compounds. We have demonstrated t...

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Autors principals: Sadique, Azwana R., Gregory, Elizabeth A., Brennessel, William W., Holland, Patrick L.
Format: Artigo
Idioma:Inglês
Publicat: 2007
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Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC2548314/
https://ncbi.nlm.nih.gov/pubmed/17564444
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja069199r
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