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Proton-Coupled Electron Transfer Reactivity Controls Iron Versus Sulfur Oxidation in Nonheme Iron Thiolate Complexes

Reaction of the 5-coordinate Fe(II)(N(4)S) complexes, [Fe(II)(iPr(3)TACN)(abt(x))](OTf) (abt = aminobenzenethiolate, X = H, CF(3)) with a one-electron oxidant and an appropriate base leads to net H-atom loss, generating new Fe(III)(iminobenzenethiolate) complexes that were characterized by single-cr...

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Bibliografiska uppgifter
I publikationen:Inorg Chem
Huvudupphovsmän: Gordon, Jesse B., McGale, Jeremy P., Siegler, Maxime A., Goldberg, David P.
Materialtyp: Artigo
Språk:Inglês
Publicerad: 2021
Ämnen:
Länkar:https://ncbi.nlm.nih.gov/pmc/articles/PMC8139613/
https://ncbi.nlm.nih.gov/pubmed/33872005
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.inorgchem.0c03779
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