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Dioxygen-Derived Nonheme Mononuclear Fe(III)(OH) Complex and Its Reactivity with Carbon Radicals

A new tetradentate, monoanionic, mixed N/O donor ligand (BNPA(Ph2)O(−)) with second coordination sphere H-bonding groups has been synthesized for stabilization of terminal Fe(III)(OH)(X) complexes. The complex [Fe(II)(BNPA(Ph2)O)(OTf)] (1) reacts with O(2) to give a mononuclear terminal Fe(III)(OH)...

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Publicat a:J Am Chem Soc
Autors principals: Yadav, Vishal, Gordon, Jesse B., Siegler, Maxime A., Goldberg, David P.
Format: Artigo
Idioma:Inglês
Publicat: 2019
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC8006860/
https://ncbi.nlm.nih.gov/pubmed/31244183
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b03329
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