A Thioether-Ligated Cupric Superoxide Model with Hydrogen Atom Abstraction Reactivity

The central role of cupric superoxide intermediates proposed in hormone and neurotransmitter biosynthesis by noncoupled binuclear copper monooxygenases like dopamine-β-monooxygenase has drawn significant attention to the unusual methionine ligation of the Cu(M) (“Cu(B)”) active site characteristic o...

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Publicat a:J Am Chem Soc
Autors principals: Bhadra, Mayukh, Transue, Wesley J., Lim, Hyeongtaek, Cowley, Ryan E., Lee, Jung Yoon C., Siegler, Maxime A., Josephs, Patrick, Henkel, Gerald, Lerch, Markus, Schindler, Siegfried, Neuba, Adam, Hodgson, Keith O., Hedman, Britt, Solomon, Edward I., Karlin, Kenneth D.
Format: Artigo
Idioma:Inglês
Publicat: 2021
Matèries:
Article
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC8023764/
https://ncbi.nlm.nih.gov/pubmed/33684290
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.1c00260
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