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Intramolecular Hydrogen Bonding Enhances Stability and Reactivity of Mononuclear Cupric Superoxide Complexes

[(L)Cu(II)(O(2)(•−))](+) (i.e., cupric-superoxo) complexes, as the first and/or key reactive intermediates in (bio)chemical Cu-oxidative processes, including in the monooxygenases PHM and DβM, have been systematically stabilized by intramolecular hydrogen bonding within a TMPA ligand-based framework...

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Podrobná bibliografie
Vydáno v:J Am Chem Soc
Hlavní autoři: Bhadra, Mayukh, Lee, Jung Yoon C., Cowley, Ryan E., Kim, Sunghee, Siegler, Maxime A., Solomon, Edward I., Karlin, Kenneth D.
Médium: Artigo
Jazyk:Inglês
Vydáno: 2018
Témata:
On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC6217813/
https://ncbi.nlm.nih.gov/pubmed/29957998
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.8b04671
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