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Copper-Catalyzed Functionalization of Benzylic C–H Bonds with NFluorobenzenesulfonimide (NFSI): Switch from C–N to C–F Bond Formation Promoted by a Redox Buffer and Brønsted Base

A copper catalyst in combination with N-fluorobenzenesulfonimide (NFSI) has been reported to functionalize benzylic C–H bonds to the corresponding benzylic sulfonimides via C–N coupling. Here, we reported a closely related Cu-catalyzed method with NFSI that instead leads to C–F coupling. This switch...

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Detaylı Bibliyografya
Yayımlandı:Org Lett
Asıl Yazarlar: Buss, Joshua A., Vasilopoulos, Aristidis, Golden, Dung L., Stahl, Shannon S.
Materyal Türü: Artigo
Dil:Inglês
Baskı/Yayın Bilgisi: 2020
Konular:
Online Erişim:https://ncbi.nlm.nih.gov/pmc/articles/PMC7446155/
https://ncbi.nlm.nih.gov/pubmed/32790419
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.0c02239
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