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Highly Stereoselective Synthesis of Fused Cyclopropane-γ-Lactams via Biocatalytic Iron-Catalyzed Intramolecular Cyclopropanation

We report the development of an iron-based biocatalytic strategy for the asymmetric synthesis of fused cyclopropane-γ-lactams, which are key structural motifs found in synthetic drugs and bioactive natural products. Using a combination of mutational landscape and iterative site-saturation mutagenesi...

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Detalhes bibliográficos
Publicado no:ACS Catal
Main Authors: Ren, Xinkun, Chandgude, Ajay L., Fasan, Rudi
Formato: Artigo
Idioma:Inglês
Publicado em: 2020
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7111458/
https://ncbi.nlm.nih.gov/pubmed/32257580
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acscatal.9b05383
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