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Enantioselective Iridium-Catalyzed Allylation of Acetylenic Ketones via 2-Propanol-Mediated Reductive Coupling of Allyl Acetate: C14-C23 of Pladienolide D

Alkyne-Directed Chemo- and Enantioselectivity. Highly enantioselective catalytic reductive coupling of allyl acetate with acetylenic ketones occurs in a chemoselective manner in the presence of aliphatic or aromatic ketones. This method was used to construct C14-C23 of pladienolide D in half the ste...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Brito, Gilmar A., Jung, Woo-Ok, Yoo, Minjin, Krische, Michael J.
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6917958/
https://ncbi.nlm.nih.gov/pubmed/31490591
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201908939
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