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A regioselectivity switch in Pd-catalyzed hydroallylation of alkynes

By exploiting the reactivity of a vinyl-Pd species, we control the regioselectivity in hydroallylation of alkynes under Pd-hydride catalysis. A monophosphine ligand and carboxylic acid combination promotes 1,5-dienes through a pathway involving isomerization of alkynes to allenes. In contrast, a bis...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Ji, Ding-Wei, Hu, Yan-Cheng, Zheng, Hao, Zhao, Chao-Yang, Chen, Qing-An, Dong, Vy M.
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6598511/
https://ncbi.nlm.nih.gov/pubmed/31341584
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c9sc01527b
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