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Structures, spectroscopic properties, and dioxygen reactivity of 5- and 6-coordinate nonheme iron(II) complexes: a combined enzyme/model study of thiol dioxygenases

The synthesis of four new Fe(II)(N(4)S(thiolate)) complexes as models of the thiol dioxygenases are described. They are composed of derivatives of the neutral, tridentate ligand triazacyclononane (R(3)TACN; R = Me, iPr) and 2-aminobenzenethiolate (abt(x); X = H, CF(3)), a non-native substrate for cy...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Gordon, Jesse B., McGale, Jeremy P., Prendergast, Joshua R., Shirani-Sarmazeh, Zahra, Siegler, Maxime A., Jameson, Guy N. L., Goldberg, David P.
Formato: Artigo
Idioma:Inglês
Publicado em: 2018
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6596423/
https://ncbi.nlm.nih.gov/pubmed/30346746
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.8b08349
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