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Preparation of Chiral Allenes through Pd-Catalyzed Intermolecular Hydroamination of Conjugated Enynes: Enantioselective Synthesis Enabled by Catalyst Design

In this study, we establish that conjugated enynes undergo selective 1,4-hydroamination under Pd catalysis to deliver chiral allenes with pendant allylic amines. Several primary and secondary aliphatic and aryl-substituted amines couple with a wide range of mono- and disubstituted enynes in a nonena...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Adamson, Nathan J., Jeddi, Haleh, Malcolmson, Steven J.
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6568270/
https://ncbi.nlm.nih.gov/pubmed/31070902
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b02637
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