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Spin Interconversion of Heme-Peroxo-Copper Complexes Facilitated by Intramolecular Hydrogen-Bonding Interactions

Synthetic peroxo-bridged high-spin (HS) heme-(μ-η(2):η(1)-O(2)(2−))-Cu(L) complexes incorporating (as part of the copper ligand) intramolecular hydrogen-bond (H-bond) capabilities and/or steric effects are herein demonstrated to affect the complex’s electronic and geometric structure, notably impact...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Schaefer, Andrew W., Ehudin, Melanie A., Quist, David A., Tang, Joel A., Karlin, Kenneth D., Solomon, Edward I.
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6457345/
https://ncbi.nlm.nih.gov/pubmed/30836005
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b00118
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