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Ta(2)(+)-mediated ammonia synthesis from N(2) and H(2) at ambient temperature
In a full catalytic cycle, bare Ta(2)(+) in the highly diluted gas phase is able to mediate the formation of ammonia in a Haber–Bosch-like process starting from N(2) and H(2) at ambient temperature. This finding is the result of extensive quantum chemical calculations supported by experiments using...
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| Published in: | Proc Natl Acad Sci U S A |
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| Main Authors: | , , , |
| Format: | Artigo |
| Language: | Inglês |
| Published: |
National Academy of Sciences
2018
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| Subjects: | |
| Online Access: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6243240/ https://ncbi.nlm.nih.gov/pubmed/30352846 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1814610115 |
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