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A Reaction‐Induced Localization of Spin Density Enables Thermal C−H Bond Activation of Methane by Pristine FeC(4) (+)

The reactivity of the cationic metal‐carbon cluster FeC(4) (+) towards methane has been studied experimentally using Fourier‐transform ion cyclotron resonance mass spectrometry and computationally by high‐level quantum chemical calculations. At room temperature, FeC(4)H(+) is formed as the main ioni...

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Bibliografiska uppgifter
I publikationen:Chemistry
Huvudupphovsmän: Geng, Caiyun, Li, Jilai, Weiske, Thomas, Schwarz, Helmut
Materialtyp: Artigo
Språk:Inglês
Publicerad: John Wiley and Sons Inc. 2019
Ämnen:
Länkar:https://ncbi.nlm.nih.gov/pmc/articles/PMC6852486/
https://ncbi.nlm.nih.gov/pubmed/31268193
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/chem.201902572
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