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Pd-Catalyzed Acyl C–O Bond Activation for Selective Ring-opening of α-Methylene-β-lactones with Amines

A Pd-catalyzed ring-opening of β-lactones with various types of amines (primary, secondary and aryl) to provide β-hydroxy amides with excellent selectivity towards acyl C–O bond cleavage is reported. The utility of this protocol is demonstrated in an asymmetric kinetic resolution providing enantioen...

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Detalhes bibliográficos
Publicado no:Org Lett
Main Authors: Malapit, Christian A., Caldwell, Donald R., Sassu, Nicole, Milbin, Samuel, Howell, Amy R.
Formato: Artigo
Idioma:Inglês
Publicado em: 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5839468/
https://ncbi.nlm.nih.gov/pubmed/28375015
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.orglett.7b00494
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