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Ti-catalyzed ring-opening oxidative amination of methylenecyclopropanes with diazenes

The ring-opening oxidative amination of methylenecyclopropanes (MCPs) with diazenes catalyzed by py(3)TiCl(2)(NR) complexes is reported. This reaction selectively generates branched α-methylene imines as opposed to linear α,β-unsaturated imines, which are difficult to access via other methods. Produ...

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Détails bibliographiques
Publié dans:Chem Sci
Auteurs principaux: Beaumier, Evan P., Ott, Amy A., Wen, Xuelan, Davis-Gilbert, Zachary W., Wheeler, T. Alexander, Topczewski, Joseph J., Goodpaster, Jason D., Tonks, Ian A.
Format: Artigo
Langue:Inglês
Publié: The Royal Society of Chemistry 2020
Sujets:
Accès en ligne:https://ncbi.nlm.nih.gov/pmc/articles/PMC8159277/
https://ncbi.nlm.nih.gov/pubmed/34123005
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/d0sc01998d
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