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Catalytic Alkylation of Remote C-H Bonds Enabled by Proton-Coupled Electron Transfer
Despite significant advances in hydrogen atom transfer (HAT) catalysis,(1–5) there are currently no molecular HAT catalysts capable of homolyzing the strong N-H bonds of N-alkyl amides (Figure 1a). The motivation to develop amide homolysis protocols stems from the synthetic utility of the resulting...
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| Publicado no: | Nature |
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| Main Authors: | , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2016
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5704892/ https://ncbi.nlm.nih.gov/pubmed/27732585 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/nature19811 |
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