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EPR/ENDOR and theoretical study of the Jahn-Teller active [HIPTN(3)N]Mo(V)L complexes (L = N(−), NH)
The molybdenum trisamidoamine (TAA) complex [Mo] (=(3,5-(2,4,6-i-Pr(3)C(6)H(2))(2)C(6)H(3)NCH(2)CH(2)N)Mo) carries out catalytic reduction of N(2) to ammonia by protons and electrons at room temperature. A key intermediate in the proposed [Mo] nitrogen reduction cycle is nitrido-Mo(VI), [Mo(VI)]N: t...
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| Publicado no: | Inorg Chem |
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| Main Authors: | , , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2017
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5678948/ https://ncbi.nlm.nih.gov/pubmed/28571321 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.inorgchem.7b00364 |
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