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Formation of {[HIPTN(3)N]Mo(III)H}(−) by Heterolytic Cleavage of H(2) as Established by EPR and ENDOR Spectroscopy
MoN(2) (Mo = [(HIPTNCH(2)CH(2))(3)N]Mo, where HIPT = 3,5-(2,4,6-i-Pr(3)C(6)H(2))(2)C(6)H(3)) is the first stage in the reduction of N(2) to NH(3) by Mo. Its reaction with dihydrogen in fluid solution yields ‘MoH(2)’, a molybdenum-dihydrogen compound. In this report, we describe a comprehensive EPR a...
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| Main Authors: | , , , , |
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| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2010
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC2844792/ https://ncbi.nlm.nih.gov/pubmed/20000748 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ic902006v |
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