Spectroscopic Definition of the Cu(Z)° Intermediate in Turnover of Nitrous Oxide Reductase and Molecular Insight into the Catalytic Mechanism

Spectroscopic methods and density functional theory (DFT) calculations are used to determine the geometric and electronic structure of Cu(Z)°, an intermediate form of the Cu(4)S active site of nitrous oxide reductase (N(2)OR) that is observed in single turnover of fully reduced N(2)OR with N(2)O. El...

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Argitaratua izan da:J Am Chem Soc
Egile Nagusiak: Johnston, Esther M., Carreira, Cíntia, Dell’Acqua, Simone, Dey, Somdatta Ghosh, Pauleta, Sofia R., Moura, Isabel, Solomon, Edward I.
Formatua: Artigo
Hizkuntza:Inglês
Argitaratua: 2017
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Article
Sarrera elektronikoa:https://ncbi.nlm.nih.gov/pmc/articles/PMC5532879/
https://ncbi.nlm.nih.gov/pubmed/28228011
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b13225
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