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Spectroscopic Definition of the Cu(Z)° Intermediate in Turnover of Nitrous Oxide Reductase and Molecular Insight into the Catalytic Mechanism

Spectroscopic methods and density functional theory (DFT) calculations are used to determine the geometric and electronic structure of Cu(Z)°, an intermediate form of the Cu(4)S active site of nitrous oxide reductase (N(2)OR) that is observed in single turnover of fully reduced N(2)OR with N(2)O. El...

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Библиографические подробности
Опубликовано в: :	J Am Chem Soc
Главные авторы:	Johnston, Esther M., Carreira, Cíntia, Dell’Acqua, Simone, Dey, Somdatta Ghosh, Pauleta, Sofia R., Moura, Isabel, Solomon, Edward I.
Формат:	Artigo
Язык:	Inglês
Опубликовано:	2017
Предметы:	Article
Online-ссылка:	https://ncbi.nlm.nih.gov/pmc/articles/PMC5532879/ https://ncbi.nlm.nih.gov/pubmed/28228011 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b13225
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Spectroscopic Definition of the Cu(Z)° Intermediate in Turnover of Nitrous Oxide Reductase and Molecular Insight into the Catalytic Mechanism

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