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Spectroscopic Definition of the Cu(Z)° Intermediate in Turnover of Nitrous Oxide Reductase and Molecular Insight into the Catalytic Mechanism

Spectroscopic methods and density functional theory (DFT) calculations are used to determine the geometric and electronic structure of Cu(Z)°, an intermediate form of the Cu(4)S active site of nitrous oxide reductase (N(2)OR) that is observed in single turnover of fully reduced N(2)OR with N(2)O. El...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Johnston, Esther M., Carreira, Cíntia, Dell’Acqua, Simone, Dey, Somdatta Ghosh, Pauleta, Sofia R., Moura, Isabel, Solomon, Edward I.
Formato: Artigo
Idioma:Inglês
Publicado em: 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5532879/
https://ncbi.nlm.nih.gov/pubmed/28228011
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b13225
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