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The Mechanism of N-N Double Bond Cleavage by an Iron(II)-Hydride Complex

The use of hydride species for substrate reductions avoids strong reductants, and may enable nitrogenase to reduce multiple bonds without unreasonably low redox potentials. In this work, we explore the N=N bond cleaving ability of a high-spin iron(II) hydride dimer with concomitant release of H(2)....

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Pubblicato in:J Am Chem Soc
Autori principali: Bellows, Sarina M., Arnet, Nicholas A., Gurubasavaraj, Prabhuodeyara M., Brennessel, William W., Bill, Eckhard, Cundari, Thomas R., Holland, Patrick L.
Natura: Artigo
Lingua:Inglês
Pubblicazione: 2016
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Accesso online:https://ncbi.nlm.nih.gov/pmc/articles/PMC5499983/
https://ncbi.nlm.nih.gov/pubmed/27598037
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b04654
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