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N-heterocyclic carbene induced reductive coupling of phosphorus tribromide. Isolation of a bromine bridged P–P bond and its subsequent reactivity

The room temperature reaction of a 1 : 1 mixture of phosphorus tribromide (PBr(3)) and the N-heterocyclic carbene 1,3-bis(2,6-diisopropylphenyl)-imidazol-2-ylidene (IPr) quantitatively affords the Lewis acid–base adduct (IPr)PBr(3) (1). Interestingly, when 1 is heated between 55 and 65 °C for a peri...

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發表在:Chem Sci
Main Authors: Waters, Jordan B., Everitt, Thomas A., Myers, William K., Goicoechea, Jose M.
格式: Artigo
語言:Inglês
出版: Royal Society of Chemistry 2016
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在線閱讀:https://ncbi.nlm.nih.gov/pmc/articles/PMC5356258/
https://ncbi.nlm.nih.gov/pubmed/28451133
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c6sc02343f
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